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    Comparison of phenol removal with ozonation in jet loop reactor and bubble column
    (Elsevier Sci Ltd, 2020) Barlak, Melahat Semin; Degermenci, Nejdet; Cengiz, Ibrahim; Ozel, Handan Ucun; Yildiz, Ergun
    This study aimed to remove phenol with ozonation in a jet loop reactor (JLR) and a bubble column (BC). In the first stage of the study, the mass transfer properties of JLR were determined and superiority over BC reactors were shown, and in the second stage, these reactors were used in phenol removal studies. At the same conditions, the volumetric mass transfer coefficient of JLR was 0.540 min-1, while this value was determined as 0.246 min(-1) in the BC reactor. In phenol removal, the effects of initial phenol concentration, ozone dosage and pH on phenol and chemical oxygen demand (COD) removal were determined for both JLR and BC. While the pseudo-first rate constant for phenol removal in JLR at 221 mg/min ozone dosage was 0.1756 min(-1), this value was only calculated as 0.1157 min(-1) in the BC reactor. As a result, it has been shown that JLRs can achieve higher ozone gas transfer with lower energy consumption and perform more effective phenol and COD removal than BC reactors, especially at low pH and high ozone dosages.
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    Investigation of Mass Transfer of Ozone in Jet Loop Reactor
    (Korean Institute Chemical Engineers, 2024) Cengiz, Ibrahim; Degermenci, Nejdet; Yildiz, Ergun; Barlak, Melahat Semin
    Mass transfer of ozone in a jet loop reactor was investigated in this study. Different parameters such as ozone gas concentration, gas flow rate, circulation flow rate, and spray nozzle diameter were examined for their effect on mass transfer. In experiments with ozone gas concentrations ranging from 3.83 to 17.1 g/m3, the KLa values remained unchanged, with an average of 28.7 +/- 2.2 h-1. As the ozone gas concentration increased, the saturation values of ozone in the liquid phase also increased. Experiments were carried out with gas flow rates ranging from 50 to 250 L/h in the jet loop reactor, and increasing gas flow rates increased the KLa value up to five times. When the effect of the liquid circulation flow rate was examined for a spray nozzle diameter of 15.5 mm, increasing the flow rate from 40 L/min to 80 L/min increased the KLa value by approximately 41%. However, the power consumed per reactor volume for this process increased 8 times and reached 2.65 kW/m3. KLa values in the JLR vary between 6.1 and 37.3 h-1 depending on operating parameters and it has been concluded that it performs well compared to its counterparts.